The potential danger of radioactive waste from deep burial for future generations after reaching the surface of the earth. The role of the radiation-equivalent principle of nuclear fuel cycle waste disposal

«Radiation and Risk», 2025, vol. 34, No. 4, pp.5-17

DOI: 10.21870/0131-3878-2025-34-4-5-17

Authors

Spirin E.V. – Chief Researcher of Dep. of the Chief Radioecologist, Project “Proryv”, D. Sc., Biol.
Solomatin V.M. – Head of Dep. of the Chief Radioecologist, Project “Proryv”, C. Sc., Biol. JSC “Proryv”. Contacts: 4 Korolyov str., Obninsk, Kaluga region, Russia, 249035. Tel.: +7(484) 399-32-81; e-mail: This email address is being protected from spambots. You need JavaScript enabled to view it. .
Menyajlo A.N. – Lead. Researcher, C. Sc., Biol.
Ivanov V.K. – Scientific Advisor of NRER, Chief Radioecologist of Project “Proryv”, Chairman of RSCRP, Corresponding Member of RAS, D. Sc., Tech., Prof. A. Tsyb MRRC.
1 Joint Stock Company “Proryv”, Moscow
2 A. Tsyb MRRC, Obninsk

Abstract

An assessment of the expected effective dose (EED) and carcinogenic risks from the consumption of well water over the radioactive waste repository when radionuclides enter the environment has been carried out. Screening calculations using a simplified model of convective motion of radionuclides with pore water have shown, that when reprocessing spent nuclear fuel on the principle of radiation equivalence with uranium raw materials, the EED at the time of radionuclide release to the Earth's surface is 100 times less than when separating only fissile materials from spent nuclear fuel. 99Tc and 237Np form more than 90% of the dose in all cases with and without spent nuclear fuel processing. 129I and 79Se contribute less to the dose. The main contribution to the dose from the decay products of actinides is 237Np, which is formed during the decay of 241Am and 241Pu. The variability of dose and risk reaches three orders of magnitude, depending on the distribution coefficients between the solid and liquid phases of radionuclides. The purification of radioactive waste from separate fractions of minor actinides and fission products, as well as the geochemical properties of the rock, most significantly affect the value of EED.

Key words
expected effective dose, radioactive waste, underground repository, radiation equivalence, migration with water, distribution coefficient, rock, environmental health, public health.

References

1. Safety indicators for the safety assessment of radioactive waste disposal. IAEA-TECDOC-1372. Vienna, IAEA, 2003. 41 p.

2. Derivation of activity limits for the disposal of radioactive waste in near surface disposal facilities. IAEA-TECDOC-1380. Vienna, IAEA, 2003. 150 p.

3. Considering timescales in the post-closure safety of geological disposal of radioactive waste. NEA OECD-6424. Paris, NEA, 2009. 163 p.

4. The safety case and safety assessment for the disposal of radioactive waste. IAEA Specific Safety No. SSG-23. Vienna, IAEA, 2012. 140 p.

5. Review of foreign practices of spent nuclear fuel and radioactive waste disposal. Eds.: I.I. Linge and Yu.D. Polyakov. Moscow, Publ. house “Komtekhprint”, 2015. 208 p. (In Russian).

6. Melikhova E.M. Public perception of the environmental impact of nuclear industry enterprises. Radioeco-logical situation in the regions where Rosatom enterprises are located. Eds.: I.I. Linge and I.I. Kryshev. Moscow, “SAM Polygraphist”, 2015, pp. 269-296. (In Russian).

7. Adamov E.O., Ganev I.H. Ecologically impeccable nuclear power engineering. Moscow, N.A. Dollezhal NIKIET, 2007. 145 p. (In Russian).

8. Adamov E.O., Gabaraev B.A., Ganev I.Kh., Lopatkin A.V., Muratov V.G., Orlov V.V. Development potential and the possibility of achieving radiation equivalence of uranium and waste in scenarios for the development of promising nuclear energy. Preprint of FSUE NIKIET ET-04/68. Moscow, FSUE NIKIET, 2004. 22 p. (In Russian).

9. Adamov E.O., Mochalov Yu.S., Rachkov V.I., Khomyakov Yu.S., Shadrin A.Yu., Kashcheev V.A., Khaperskaya A.V. Reprocessing of spent nuclear fuel and recycling of nuclear materials in two-component nuclear power engineering. Atomnaya energiya – Atomic Energy, 2021, vol. 130, no. 1, pp. 28-34. (In Russian).

10. Radiological safety of the public in two-component nuclear power engineering. Ed.: V.K. Ivanov. Obninsk, 2023. 256 p. (In Russian).

11. Ivanov V.K. Nuclear power plants based on fast neutron reactors: the final solution to the problem of spent nuclear fuel and radioactive waste. Byulleten Atomproma – Bulletin of Atomprom, 2024, N 1, pp. 43. (In Russian).

12. Adamov E.O., Ganev I.Kh., Lopatkin A.V., Muratov V.G., Orlov V.V. Transmutation fuel cycle in large-scale nuclear power engineering in Russia. Moscow, GUP NIKIET, 1999. 252 p. (In Russian).

13. Ivanov V.K., Lopatkin A.V., Spirin E.V., Solomatin V.M., Menyajlo A.N., Chekin S.Yu., Lovachev S.S. Achievability of radiological equivalence associated with closed nuclear fuel cycle with fast reactors: impact of uncertainty factors in scenarios of Russian nuclear power development through to 2100. Part 2. Migration of radionuclides. Radiatsiya i risk – Radiation and Risk, 2021, vol. 30, no. 3, pp. 8-20. (In Russian).

14. Ivanov V.K., Spirin E.V., Lopatkin A.V., Menyajlo A.N., Chekin S.Yu., Solomatin V.M., Korelo A.M., Tumanov K.A. Correlation between potential radiation-induced carcinogenic risks associated with WWER-1000 spent nuclear fuel and BREST-1200 radiation waste in case of annual generation of 1 GW of electricity. Part 2. Radiological migration equivalence. Radiatsiya i risk – Radiation and Risk, 2022, vol. 31, no. 2, pp. 5-20. (In Russian).

15. Spirin E.V., Solomatin V.M., Menyajlo A.N., Ivanov V.K. Potential biological hazard of Cm isotopes in deep burial. Radiatsiya i risk – Radiation and Risk, 2024, vol. 33, no. 3, pp. 5-17. (In Russian).

16. Kapyrin I.V., Boldyrev K.A. Transport process modeling assuming chemical interactions in the GeRa software. Radioactivnye otkhody – Radioactive Waste, 2024, no. 1 (26), pp. 84-94. (In Russian).

17. Prokhorov V.M. Migration of radioactive contamination in soils (physico-chemical mechanisms and modeling). Ed.: R.M. Aleksakhin. Moscow, Energoizdat, 1981. 99 p. (In Russian).

18. Konovalova L.N., Zinovieva L.M., Ghukasyan T.K. Formation physics. The training manual. Stavropol, 2016. 120 p. (In Russian).

19. Sheppard M.I., Thibault D.H. Default soil solid/liquid partition coefficients, Kds, for four major soil types: a compendium. Health Phys., 1990, vol. 59, no. 4, pp. 471-482.

20. Quantification of radionuclide transfer in terrestrial and freshwater environments for radiological assessments. IAEA-TECDOC-1616. Vienna, IAEA, 2009. 625 p.

21. Ivanov V.K., Spirin E.V., Lopatkin A.V., Menyajlo A.N., Chekin S.Yu., Solomatin V.M., Korelo A.M., Tumanov K.A. Correlation between potential radiation-induced carcinogenic risks associated with WWER-1000 spent nuclear fuel and BREST-1200 radiation waste in case of annual generation of 1 GW of electricity. Part 1. Radiological equivalence. Radiatsiya i risk – Radiation and Risk, 2022, vol. 31, no. 1, pp. 5-14. (In Russian).

22. Basic Sanitary Rules for Radiation Safety (OSPORB-99/2010). Health regulations. SP 2.6.1.2612-10. Moscow, Center for Sanitary and Epidemiological Rationing, Hygienic Certification of Russian Ministry of Health, 2010. (In Russian).

23. Strategy for the development of radioactive waste deep disposal facility. Radioactivnye otkhody – Radioactive Waste, 2018, no. 2 (3), pp. 114-1120. (In Russian).

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